Supporting data for Temperature-dependent thermal conductivity of MBE-grown epitaxial SrSnO₃ films

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2021-12-14
2023-06-29

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2023-07-05

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Supporting data for Temperature-dependent thermal conductivity of MBE-grown epitaxial SrSnO₃ films

Published Date

2023-11-06

Author Contact

Wang, Xiaojia
wang4940@umn.edu

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Experimental Data
Simulation Data

Abstract

This work studies the temperature-dependent thermal properties of a single crystalline SSO thin film prepared with hybrid molecular beam epitaxy. By combining time-domain thermoreflectance and Debye–Callaway modeling, physical insight into thermal transport mechanisms is provided. At room temperature, the 350-nm SSO film has a thermal conductivity of 4.4 W m¯¹ K¯¹ , ∼60% lower than those of other perovskite oxides (SrTiO₃, BaSnO₃) with the same ABO₃ structural formula. This difference is attributed to the low zone-boundary frequency of SSO, resulting from its distorted orthorhombic structure with tilted octahedra. At high temperatures, the thermal conductivity of SSO decreases with temperature following a ∼T ¯⁰∙⁵⁴ dependence, weaker than the typical T¯¹ trend dominated by the Umklapp scattering. Corresponding author for STEM data is K. Andre Mkhoyan. Corresponding author for film growth and XRD data is Bharat Jalan. Corresponding author for TDTR data is Xiaojia Wang.

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A single excel file containing all raw data for plots (outputs), including the main paper and the Supplementary Material, following the order of figure numbers. Archive of data included in .csv format.

Referenced by

Chi Zhang, Fengdeng Liu, Silu Guo, Yingying Zhang, Xiaotian Xu, K. Andre Mkhoyan, Bharat Jalan, Xiaojia Wang; Temperature-dependent thermal conductivity of MBE-grown epitaxial SrSnO₃ films. Appl. Phys. Lett. 24 July 2023; 123 (4): 042201.
https://doi.org/10.1063/5.0156367

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Funding information

National Science Foundation through the MRSEC program (Award No. DMR-2011401)
NSF (Award No. CEBT-2226579)
Air Force Office of Scientific Research (AFOSR) through Grant Nos. FA9550-21-1-0025, and FA9550-23-1-0247
National Nanotechnology Coordinated Infrastructure (NNCI) under Award Number ECCS-2025124

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Suggested citation

Zhang, Chi; Liu, Fengdeng; Guo, Silu; Zhang, Yingying; Xu, Xiaotian; Mkhoyan, Andre; Jalan, Bharat; Wang, Xiaojia. (2023). Supporting data for Temperature-dependent thermal conductivity of MBE-grown epitaxial SrSnO₃ films. Retrieved from the University Digital Conservancy, https://doi.org/10.13020/tmn3-ds92.
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README_APL_T-depSSO.pdfDescription of data511.53 KB
SSO_source_AllData_11_02_2023.xlsxAll the data corresponding to the figures in the main paper and supplementary material172 KB
AllData_Archive.zipArchival format of all data (11 .csv)156.3 KB

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