Anderson, Nathan2021-09-242021-09-242021-06https://hdl.handle.net/11299/224495University of Minnesota M.S.Ch.E. thesis. June 2021. Major: Chemical Engineering. Advisor: Zhihua Xu. 1 computer file (PDF); ix, 116 pages.Charge carrier dynamics and ion migration are attributed to the current-voltage hysteresis in perovskite solar cells (PSCs). This study implements a drift-diffusion model in Python to simulate the characteristic current-voltage scans for realistic device architectures. The novel work in this research involve the integration of a transfer-matrix optical model to the drift-diffusion model with ion migration, the implementation of a Radau 5th order solver to the method of lines, and a demonstration that standard Python libraries can handle stiff systems of differential algebraic equations. A comparative analysis with published works was conducted to validate the algorithm. It was found that the simulation was able to capture fast carrier dynamics under a variety of experimental conditions. Lastly, it is shown that the model captures physically relevant trends in PSCs.enDrift-DiffusionHysteresisIon MigrationPerovskite Solar CellPythonTransfer-matrixThesis or Dissertation